Dual-arm Z-scan technique to extract dilute solute nonlinearities from solution measurements

Dual-arm Z-scan technique to extract dilute solute nonlinearities from solution measurements

We present a technique in which small solute nonlinearities may be extracted from large solvent signals by performing simultaneous Z-scans on two samples (solvent and solution). By using a dual-arm Z-scan apparatus with identical arms, fitting error in determining the solute nonlinearity is reduced because the irradiance fluctuations are correlated for both the solvent and solution measurements...

Z-Scan Measurements of Optical Nonlinearities

Time-resolved Z-scan measurements of optical nonlinearities

We introduce a temporal delay in one beam of the two-color Z-scan apparatus, which measures nondegenerate nonlinear absorption and nondegenerate nonlinear refraction. This technique allows us to time resolve separately the sign and the magnitude of the nonlinear absorption and refraction at frequency p that are due to the presence of a strong excitation at frequency oe. For example, in semicond...

Nonlinear refractive index measurement on pure and Nd doped YAG ceramic by dual arm Z-scan technique

Transparent ceramics gain much attention as an alternative medium for high power ultra-short lasers because of its superior thermal properties over single crystals. Measurement of nonlinear refractive index is essential to understand the limit of such material for ultra-short laser generation. Dual arm Z-scan technique was employed to measure n2 for single crystal and ceramic at the same time t...

Measurement of nondegenerate nonlinearities using a two-color Z scan.

A simple dual-wavelength (two-color) Z-scan geometry is demonstrated for measuring nonlinearities at frequency omega(p) owing to the presence of light at omega(e). This technique gives the nondegenerate two-photon absorption (2PA) coefficient beta(omega(p); omega(e)) and the nondegenerate nonlinear refractive index n(2)(omega(p); omega(e)), i.e., cross-phase modulation. We demonstrate this tech...